I stumbled on this problem in the wake of the discussion https://math.stackexchange.com/a/3553902/198592
Can you make sense of the equation in the question involving the harmonic number with a rational index $H_{\frac{2}{3} k}$ although the series is not convergent?
Hint: find the generating function of $g(z) = \sum_{k=1}^{\infty}z^k H_{\frac{2 k}{3}}$ and interpret the sum as the limit $z\to -1$.