I'm not sure how to evaluate the sum $\sum_{d|n}\tau(d)\mu(d)$, since it is also not a convolution.
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3Still, $\tau(d)\mu(d)$ is a multiplicative function of $d$, so your sum is a multiplicative function of $n$. Can you evaluate it when $n$ is a prime power? – Greg Martin Jun 26 '14 at 01:14
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Assume $n \gt 1$.
If $n = \prod_{i=1}^{\omega(n)} p_i^{e_i}$ with $p_i$ prime (and distinct from $p_j$) and $e_i \gt 0$, then similar to the proof that $\sum_{d|n} \mu(d) = 0$ we get that
$$\sum_{d|n} \tau(d) \mu(d) = \binom{\omega(n)}{r} (-1)^r 2^r = (1-2)^{\omega(n)} = (-1)^{\omega(n)}$$
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