After answering this question, I decided to change it a bit (had some free time), and turned it into a Gross-Pitaevskii equation. Suddenly, the code that used to work now gives the error message:
CoefficientArrays::poly: "1/2 (-ψ$6110-ψ$6111)+ψ (1- 1/Sqrt[1+x$6089^2+y$6090^2]+0.1 Abs[ψ]^2) is not a polynomial.
I tried changing the potential for the Harmonic Oscillator, but still no use.
My code:
ClearAll["Global`*"];
g = 0.1;
X = 5;
V[x_, y_] := 1/2 (x^2 + y^2);
ini[x_, y_] := Exp[-(x^2 + y^2)];
bc = ψ[x, y] ==
ini[x, y] /. {{x -> X}, {x -> -X}, {y -> X}, {y -> -X}};
sys = {-1/
2 (D[ψ[x, y], {x, 2}] +
D[ψ[x, y], {y, 2}]) + (V[x, y] +
g Abs[ψ[x, y]^2]) ψ[x, y] == Etr ψ[x, y], bc};
sol = ParametricNDSolveValue[
sys, ψ, {x, -X, X}, {y, -X, X}, {Etr}];
Plot3D[Abs[sol[1][x, y]], {x, -X, X}, {y, -X, X}, PlotRange -> All]
If I set g=0, I get some good results. Any other value and I get the error message.
Can anyone explain what's going on? How can it be fixed?

"FiniteElement"method can't handle nonlinear equations at the moment… – xzczd May 26 '17 at 02:02sol? I mean, try executing e.g.sol[1]. – xzczd May 26 '17 at 03:15