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Microsoft Lync allows to select the primary communication device so I can switch between my USB headset and PC speaker/mic. But the settings is used for new calls only. Is there a possibility to change the communication device for a call in progress?

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In Lync 2010, it seems to be possible to select a different audio or video device.

But the settings have no impact until you end the call, and re-establish it.

So, practically, NO.