Here's an option using asymptote instead of pgfplots. Compile with pdflatex -shell-escape.
\documentclass{standalone}
\usepackage{asypictureB}
\begin{document}
\begin{asypicture}{name=spherical-harmonic-L-M-4-3}
import graph3;
import palette;
size3(200,200,200);
currentprojection=orthographic(4,1,1);
//Parametric function R^2 --> R^3 for drawing the sphere
real R=1;
triple f( pair t ) {
return (
R*sin(t.y)*cos(t.x),
R*sin(t.y)*sin(t.x),
R*cos(t.y)
);
}
//Parametric function R^3 --> R^1 for coloring the sphere; normalization is not important.
int M = 3;
//int L = 4; Not actually used, but good for note-taking.
real PLM(real x){
return -105*x*(1-x^2)^1.5;
}
real SphHarm(triple v){
real r = v.x^2+v.y^2+v.z^2;
real costheta = v.z/r;
real cosphi = v.x/r;
real sinphi = v.y/r;
pair phase = (v.x + I*v.y)^M; //phase is complex number, phase.x is real part, phase.y is imaginary part
return phase.x*PLM(costheta);
}
//Create sphere surface
surface s=surface(f,(0,0),(2pi,2pi),100,Spline);
//Map colors onto surface
pen p1 = opacity(0.5)+red;
pen p2 = opacity(0.5)+white;
pen p3 = opacity(0.5)+blue;
s.colors(palette(s.map(SphHarm),Gradient(p1,p2,p3) )); //Gradient pallete interpolates between different colors
//Draw the surface
draw(s);
//Draw Axes
pen thickblack = gray+0.5;
real axislength = 1.25;
draw(L=Label("$x$",black, position=Relative(1.1), align=SW), O--axislength*X,thickblack, Arrow3);
draw(L=Label("$y$",black, position=Relative(1.1), align=E), O--axislength*Y,thickblack, Arrow3);
draw(L=Label("$z$",black, position=Relative(1.1), align=N), O--axislength*Z,thickblack, Arrow3);
\end{asypicture}
\end{document}

Some notes:
- I colored the sphere's surface based on the real part of the spherical harmonic.
- I used an explicit function to do the coloring for me, rather than a data table To change the spherical harmonic, edit
L and M, and PLM, which is the associated legendre polynomial. (Unfortunately, asymptote does not have a built-in library for these to my knowledge.)
If this is appealing to you and you want to learn more about asymptote, I recommend Charles Staats' asymptote tutorial
\addplot3 tablewith suitablex expr,y expr, andz expr, compare section "44.3.2 Reading Coordinates From Tables". If you encounter problems with the approach, you can post what you achieved here and we will assist you. – Christian Feuersänger Jul 26 '15 at 09:25