You should use FrobeniusNumber instead of FrobeniusSolve, since it serves this purpose
The Frobenius number of $a_{1}, ... a_{n}$,.is the largest integer b for which the Frobenius equation $a_{1} x_{1}+ ... a_{n} x_{n} = k$ has no non-negative integer solutions. The $a_{i}$ must be positive integers.
FrobeniusNumber[{6, 9, 20}]
43
Nevertheless you can still get the result playing with FrobeniusSolve, there might be many possible ways, let's point out one of them using Cases with an appropriate replacement rule e.g.
Max @ Cases[ Table[{ k, FrobeniusSolve[{6, 9, 20}, k] != {}}, {k, 100}], {a_, False} -> a]
43
In case of not knowing FrobeniusNumber, one can get an idea also with Reduce or Solve although these ways are not recommended for diophantine equations, see e.g. Finding the number of solutions to a diophantine equation.
FrobeniusNumber[{6, 9, 20}]. – Jacob Akkerboom May 28 '13 at 20:53FrobeniusSolve[{12, 16, 20, 27}, 88]andFrobeniusSolve[{12, 16, 20, 27}, 90]both find non-negative solutions whereas the Frobenius number of this series is supposed to beFrobeniusNumber[{12, 16, 20, 27}]==89? – Sjoerd C. de Vries May 28 '13 at 21:27Resolve[Exists[n, n >= 1 && ForAll[k, Implies[k > n, Exists[{x, y, z}, x >= 0 && y >= 0 && z >= 0 && {6, 9, 20}.{x, y, z} == k]]]], Integers]. I would not be surprised if it takes around infinitely long to resolve this though. – Daniel Lichtblau May 28 '13 at 21:43Table[ {iiii, FrobeniusSolve[{12, 16, 20, 27}, iiii, 1]}, {iiii, 500}] // Column. The point is that for iiii>89, there is always a solution. We may also not have a solution for iiii=85, but 89 is the largest number for which we have no solution. – Jacob Akkerboom May 28 '13 at 22:17